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Development of mobile miniature natural gas liquefiers

Yanxing ZHAO, Maoqiong GONG, Haocheng WANG, Hao GUO, Xueqiang DONG

《能源前沿（英文）》 2020年第14卷第4期页码 667-682 doi: 10.1007/s11708-020-0695-y

摘要： With increasing consumption of natural gas (NG), small NG reservoirs, such as coalbed methane and oil field associated gas, have recently drawn significant attention. Owing to their special characteristics (e.g., scattered distribution and small output), small-scale NG liquefiers are highly required. Similarly, the mixed refrigerant cycle (MRC) is suitable for small-scale liquefaction systems due to its moderate complexity and power consumption. In consideration of the above, this paper reviews the development of mobile miniature NG liquefiers in Technical Institute of Physics and Chemistry (TIPC), China. To effectively liquefy the scattered NG and overcome the drawbacks of existing technologies, three main improvements, i.e., low-pressure MRC process driven by oil-lubricated screw compressor, compact cold box with the new designed heat exchangers, and standardized equipment manufacturing and integrated process technology have been made. The development pattern of “rapid cluster application and flexible liquefaction center” has been eventually proposed. The small-scale NG liquefier developed by TIPC has reached a minimum liquefaction power consumption of about 0.35 kW·h/Nm . It is suitable to exploit small remote gas reserves which can also be used in boil-off gas reliquefaction and distributed peak-shaving of pipe networks.

关键词： natural gas mobile miniature liquefiers mixed refrigerant cycle vapor liquid equilibrium heat transfer

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Simulation on refrigerant flow in adiabatic capillary tube

WANG Meixia, LIU Cunfang, ZHOU Qiangtai

《机械工程前沿（英文）》 2008年第3卷第3期页码 332-336 doi: 10.1007/s11465-008-0054-x

摘要： This paper proposes a new mathematical model to calculate flow characteristics of the adiabatic capillary tube, which is aimed at solving problems existing in some earlier models. The Stocker’s model was modified with consideration of various effects due to sub-cooling, area concentration, and rolling diameter. The new model can be used not only for R22, but also for its substitutes such as R410A and R407C. A comparison of simulation results of the modified model with those in literature showed that the errors are within 10%. The flow characteristics are finally analyzed.

关键词： mathematical diameter literature sub-cooling adiabatic capillary

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Energy systems engineering: methodologies and applications

Pei LIU, Efstratios N. PISTIKOPOULOS, Zheng LI

《能源前沿（英文）》 2010年第4卷第2期页码 131-142 doi: 10.1007/s11708-010-0035-8

摘要： Energy systems are the major contributor to ever-increasing primary energy consumption and consequent greenhouse gas emissions. To tackle these critical problems, planning and design of energy systems needs to be improved towards a more efficient, cost-effective, and environmentally benign direction. However, although there are many technical choices available, they are often developed separately by their own technical communities and driven by their specific interest, thus methods and experience obtained in planning and design of a certain type of energy systems are usually not applicable to other types of energy systems. Energy systems engineering provides a generic methodological framework to facilitate the planning and design of energy systems and to produce integrated solutions to real-life complex energy problems via a systematic approach.In this paper, we present an overview of key methodologies of energy systems engineering, covering superstructure based modelling, mixed-integer programming, multi-objective optimization, optimization under uncertainty, and life-cycle assessment. Applications of these methodologies in polygeneration energy systems design, hydrogen infrastructure planning, and design of energy systems in commercial buildings are provided to demonstrate the capability of these methodologies.

关键词： energy systems engineering superstructure mixed-integer programming multi-objective optimization optimization under uncertainty life-cycle assessment

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Boiling heat transfer correlations for refrigerant mixtures flowing inside micro-fin tubes

ZHANG Xiaoyan, ZHANG Xingqun, CHEN Yunguang, YUAN Xiuling

《能源前沿（英文）》 2008年第2卷第4期页码 489-493 doi: 10.1007/s11708-008-0110-6

摘要： Based on experimental results of ternary non-azeotropic refrigerant mixture R417A flowing and boiling in one smooth and two internally grooved horizontal tubes with different geometrical parameters, a boiling heat transfer correlations was developed for refrigerant mixtures flowing inside micro-fin tubes by applying the enhancement factor in the present modified-Kattan model which was modified by the experimental data of R417A in a smooth tube. The comparison between the calculation and the experimental results indicates that the prediction by the present correlations is in good agreement with the experiment of refrigerant mixtures inside different micro-fin tubes with a standard deviation of ± 30% for vapor qualities below 80%.

关键词： comparison micro-fin calculation transfer prediction

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Iteration framework for solving mixed lubrication computation problems

《机械工程前沿（英文）》 2021年第16卷第3期页码 635-648 doi: 10.1007/s11465-021-0632-8

摘要： The general discrete scheme of time-varying Reynolds equation loses the information of the previous step, which makes it unreasonable. A discretization formula of the Reynolds equation, which is based on the Crank–Nicolson method, is proposed considering the physical message of the previous step. Gauss–Seidel relaxation and distribution relaxation are adopted for the linear operators of pressure during the numerical solution procedure. In addition to the convergent criteria of pressure distribution and load, an estimation framework is developed to investigate the relative error of the most important term in the Reynolds equation. Smooth surface with full contacts and mixed elastohydrodynamic lubrication is tested for validation. The asperity contact and sinusoidal wavy surface are examined by the proposed discrete scheme. Results show the precipitous decline in the boundary of the contact area. The relative error suggests that the pressure distribution is reliable and reflects the accuracy and effectiveness of the developed method.

关键词： mixed lubrication discretization formula relative error Reynolds equation asperity

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Perspective of mixed matrix membranes for carbon capture

Shinji Kanehashi, Colin A. Scholes

《化学科学与工程前沿（英文）》 2020年第14卷第3期页码 460-469 doi: 10.1007/s11705-019-1881-5

摘要： Polymeric membrane-based gas separation has found wide applications in industry, such as carbon capture, hydrogen recovery, natural gas sweetening, as well as oxygen enrichment. Commercial gas separation membranes are required to have high gas permeability and selectivity, while being cost-effective to process. Mixed matrix membranes (MMMs) have a composite structure that consists of polymers and fillers, therefore featuring the advantages of both materials. Much effort has been made to improve the gas separation performance of MMMs as well as general membrane properties, such as mechanical strength and thermal stability. This perspective describes potential use of MMMs for carbon capture applications, explores their limitations in fabrication and methods to overcome them, and addresses their performance under industry gas conditions.

关键词： membranes polymeric mixed matrix impurities

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new regeneration approach to cation resins with aluminum salts: application of desalination by its mixed

Zhigang LIU, Shaomin ZHU, Yansheng LI

《环境科学与工程前沿（英文）》 2012年第6卷第1期页码 45-50 doi: 10.1007/s11783-010-0262-6

摘要： A novel method for the regeneration of cation exchange resins by aluminum (Al) salts was investigated in order to improve the regeneration efficiency of resins and reduce the dosage of regenerant. The influences of Al concentration and the pH of regeneration solution on resin transformation had been studied. The desalination experiments were carried out to evaluate the characteristics of the Al form resins. Experimental results showed that the regeneration rate of resins was strictly dependent on Al concentration and the pH of the solution. Compared to the conventional regeneration method, the Al form mixed bed exhibited the same desalination capability as the H form mixed bed (MB), and the total organic carbon (TOC) removal was up to 90%, clearly higher than that of the H form. Al salt solution could be utilized repeatedly to regenerate Al form resins.

关键词： aluminum (Al) form resins desalination mixed bed (MB) regeneration

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characteristics and daily fluctuations of microplastics throughout wastewater treatment plants with mixed

《环境科学与工程前沿（英文）》 2022年第16卷第1期页码 6-6 doi: 10.1007/s11783-021-1440-4

摘要：

• MPs were analyzed throughout three WWTPs with mixed domestic–industrial influents.

关键词： Microplastic Wastewater treatment plant Mixed domestic-industrial influent Characteristic Daily fluctuation

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Scrap Iron Filings assisted nitrate and phosphate removal in low C/N waters using mixed microbial culture

《环境科学与工程前沿（英文）》 2021年第15卷第4期 doi: 10.1007/s11783-020-1358-2

摘要：

• Microbes enhance denitrification under varying DO concentrations and SIF dosages.

关键词： Scrap iron filing Nitrate removal Phosphate removal Mixed culture denitrification Zero valent iron

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A comparison of production system life cycle models

Rajesh ATTRI, Sandeep GROVER

《机械工程前沿（英文）》 2012年第7卷第3期页码 305-311 doi: 10.1007/s11465-012-0332-5

摘要：

Companies today need to keep up with the rapidly changing market conditions to stay competitive. The main issues in this paper are related to a company’s market and its competitors. The prediction of market behavior is helpful for a manufacturing enterprise to build efficient production systems. However, these predictions are usually not reliable. A production system is required to adapt to changing markets, but such requirement entails higher cost. Hence, analyzing different life cycle models of the production system is necessary. In this paper, different life cycle models of the production system are compared to evaluate the distinctive features and the limitations of each model. Furthermore, the difference between product life cycle and production life cycle is summarized, and the effect of product life cycle on production life cycle is explained. Finally, a production system life cycle model, along with key activities to be performed in each stage, is proposed specifically for the manufacturing sector.

关键词： production system life cycle model product

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Fluoride ions adsorption from water by CaCO enhanced Mn–Fe mixed metal oxides

《化学科学与工程前沿（英文）》 2023年第17卷第2期页码 236-248 doi: 10.1007/s11705-022-2193-8

摘要： Novel CaCO₃-enhanced Mn–Fe mixed metal oxides (CMFC) were successfully prepared for the first time by a simple-green hydrothermal strategy without any surfactant or template combined with calcination process. These oxides were then employed as an adsorbent for adsorptive removal of excess fluoride ions. The adsorbent was characterized by SEM, XPS, XRD, FTIR, and BET analysis techniques. The adsorption property of CMFC toward fluoride ion was analyzed by batch experiments. In fact, CMFC exhibited adsorption capacity of 227.3 mg∙g^‒1 toward fluoride ion. Results showed that ion exchange, electrostatic attraction and chemical adsorption were the main mechanism for the adhesion of large amount of fluoride ion on the CMFC surface, and the high adsorption capacity responded to the low pH of the adsorption system. When the fluoride ion concentration was increased from 20 to 200 mg∙L^‒1, Langmuir model was more in line with experimental results. The change of fluoride ion adsorption with respect to time was accurately described by pseudo-second-order kinetics. After five cycles of use, the adsorbent still maintains a performance of 70.6% of efficiency, compared to the fresh adsorbent. Therefore, this material may act as a potential candidate for adsorbent with broad range of application prospects.

关键词： mesoporous materials metal oxides fluoride ion adsorption mechanism

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Optimization and modeling of biohydrogen production by mixed bacterial cultures from raw cassava starch

Shaojie Wang,Zhihong Ma,Ting Zhang,Meidan Bao,Haijia Su

《化学科学与工程前沿（英文）》 2017年第11卷第1期页码 100-106 doi: 10.1007/s11705-017-1617-3

摘要： The production of bio-hydrogen from raw cassava starch via a mixed-culture dark fermentation process was investigated. The production yield of H was optimized by adjusting the substrate concentration and the microorganism mixture ratio. A maximum H yield of 1.72 mol H /mol glucose was obtained with a cassava starch concentration of 10 g/L to give a 90% utilization rate. The kinetics of the substrate utilization and of the generation of both hydrogen and volatile fatty acids were also investigated. The substrate utilization follows pseudo first order reaction kinetics, whereas the production of both H and the VFAs correlate with the Gompertz equation. These results show that cassava is a good candidate for the production of biohydrogen.

关键词： cassava biohydrogen mixed cultures kinetics

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Investigation of polyhydroxyalkanoates (PHAs) biosynthesis from mixed culture enriched by valerate-dominant

Jiuxiao Hao, Xiujin Wang, Hui Wang

《环境科学与工程前沿（英文）》 2017年第11卷第1期 doi: 10.1007/s11783-017-0896-8

摘要： Valerate-hydrolysate enriched culture showed great ability to produce 3HV and 3H2MV. Valerate-hydrolysate enriched culture had more in the community. Mixed iso-/n-valerate was effective at balancing microbial growth and PHAs synthesis. Co-substrates of valerate and propionate raised the fraction of 3HV and 3H2MV. The production of polyhydroxyalkanoates (PHAs) with a high fraction of 3-hydroxyvalerate (3HV) and 3-hydroxy-2-methylvalerate (3H2MV) from mixed culture enriched by valerate-dominant hydrolysate was evaluated in this study. After long-term enrichment, the culture showed strong ability to synthesize 3HV and 3H2MV, even with acetate-dominant substrate. The ultilization of single or mixed iso-/n-valerate by the enriched culture showed that the mixture of iso-valerate and n-valerate was more efficient substrate than any single in terms of balancing microbial growth and PHAs synthesis. Besides, through comparing the kinetics and stoichiometry of the tests supplying valerate and propionate, the enriched culture with equivalent valerate and propionate (1:1 molar ratio) exhibited superior PHAs production performances to pure valerate or propionate, attaining more than 70 mol% of 3HV and 3H2MV. The above findings reveal that valerate-dominant hydrolysate is a kind of suitable substrate to enrich PHAs producing culture with great capability to synthesize 3HV and 3H2MV monomers, thus improving product properties than pure poly(3-hydroxybutyrate) (P3HB); also 3HV and 3H2MV production behaviors can be regulated by the type of odd-carbon VFAs in the substrate.

关键词： Polyhydroxyalkanoates (PHAs) Valerate Mixed culture 3-hydroxyvalerate (3HV) Propionate

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Abatement of mixed volatile organic compounds in a catalytic hybrid surface/packed-bed discharge plasma

Lianjie Guo, Nan Jiang, Jie Li, Kefeng Shang, Na Lu, Yan Wu

《环境科学与工程前沿（英文）》 2018年第12卷第2期 doi: 10.1007/s11783-018-1017-z

摘要： In this study, post plasma-catalysis degradation of mixed volatile organic compounds (benzene, toluene, and xylene) has been performed in a hybrid surface/packed-bed discharge plasma reactor with Ag-Ce/ g-Al O catalyst at room temperature. The effect of relative air humidity on mixed VOCs degradation has also been investigated in both plasma-only and PPC systems. In comparison to the plasma-only system, a significant improvement can be observed in the degradation performance of mixed VOCs in PPC system with Ag-Ce/ g-Al O catalyst. In PPC system, 68% benzene, 89% toluene, and 94% xylene were degraded at 800 J·L , respectively, which were 25%, 11%, and 9% higher than those in plasma-only system. This result can be attributed to the high catalytic activity of Ag-Ce/ g-Al O catalyst to effectively decompose O and lead to generating more reactive species which are capable of destructing the VOCs molecules completely. Moreover, the presence of Ag-Ce/ g-Al O catalyst in plasma significantly decreased the emission of discharge byproducts (NO and O ) and promoted the mineralization of mixed VOCs towards CO . Adding a small amount of water vapor into PPC system enhanced the degradation efficiencies of mixed VOCs, however, further increasing water vapor had a negative impact on the degradation efficiencies, which was primarily attributed to the quenching of energetic electrons by water vapor in plasma and the competitive adsorption of water vapor on the catalyst surface. Meanwhile, the catalysts before and after discharge were characterized by the Brunauer-Emment-Teller and X-ray photoelectron spectroscopy.

关键词： Mixed VOCs HSPBD plasma reactor Degradation Catalyst Relative humidity

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Removal of Ni(II) ions from wastewater by micellar enhanced ultrafiltration using mixed surfactants

Amar D. Vibhandik, Kumudini V. Marathe

《化学科学与工程前沿（英文）》 2014年第8卷第1期页码 79-86 doi: 10.1007/s11705-014-1407-0

摘要： Ni(II) ions were removed from aqueous waste using micellar enhanced ultrafiltration (MEUF) with a mixture of surfactants. The surfactant mixture was the nonionic surfactant Tween 80 (TW80) mixed with the anionic surfactant sodium dodecyl sulfate (SDS) in different molar ratios ranging from 0.1–1.5. The operational variables of the MEUF process such as pH, applied pressure, surfactant to metal ion ratio and nonionic to ionic surfactant molar ratio (α) were evaluated. Rejection of Ni and TW80 was 99% and 98% respectively whereas that for SDS was 65%. The flux and all resistances (fouling resistance, resistance due to concentration polarization) were measured and calculated for entire range of α respectively. A calculated flux was found to be declined with time, which was mainly attributed to concentration polarization rather than resistance from membrane fouling.

关键词： MEUF Ni (II) ions membrane resistance concentration polarization mixed surfactants